start-ver=1.4 cd-journal=joma no-vol=3 cd-vols= no-issue=1 article-no= start-page=148 end-page= dt-received= dt-revised= dt-accepted= dt-pub-year=2020 dt-pub=20200827 dt-online= en-article= kn-article= en-subject= kn-subject= en-title= kn-title=Localized-to-itinerant transition preceding antiferromagnetic quantum critical point and gapless superconductivity in CeRh0.5Ir0.5In5 en-subtitle= kn-subtitle= en-abstract= kn-abstract=A fundamental problem posed from the study of correlated electron compounds, of which heavy-fermion systems are prototypes, is the need to understand the physics of states near a quantum critical point (QCP). At a QCP, magnetic order is suppressed continuously to zero temperature and unconventional superconductivity often appears. Here, we report pressure T-c. (P)-dependent In-115 nuclear quadrupole resonance (NQR) measurements on heavy-fermion antiferromagnet CeRh0.5Ir0.5In5. These experiments reveal an antiferromagnetic (AF) QCP at P-c(AF) = 1.2 GPa where a dome of superconductivity reaches a maximum transition temperature Tc. Preceding P-c(AF), however, the NQR frequency nu(Q) undergoes an abrupt increase at P-c* = 0.8 GPa in the zero-temperature limit, indicating a change from localized to itinerant character of cerium's f-electron and associated small-to-large change in the Fermi surface. At P-c(AF) where T-c is optimized, there is an unusually large fraction of gapless excitations well below T-c that implicates spin-singlet, odd-frequency pairing symmetry. en-copyright= kn-copyright= en-aut-name=KawasakiShinji en-aut-sei=Kawasaki en-aut-mei=Shinji kn-aut-name= kn-aut-sei= kn-aut-mei= aut-affil-num=1 ORCID= en-aut-name=OkaToshihide en-aut-sei=Oka en-aut-mei=Toshihide kn-aut-name= kn-aut-sei= kn-aut-mei= aut-affil-num=2 ORCID= en-aut-name=SorimeAkira en-aut-sei=Sorime en-aut-mei=Akira kn-aut-name= kn-aut-sei= kn-aut-mei= aut-affil-num=3 ORCID= en-aut-name=KogameYuji en-aut-sei=Kogame en-aut-mei=Yuji kn-aut-name= kn-aut-sei= kn-aut-mei= aut-affil-num=4 ORCID= en-aut-name=UemotoKazuhiro en-aut-sei=Uemoto en-aut-mei=Kazuhiro kn-aut-name= kn-aut-sei= kn-aut-mei= aut-affil-num=5 ORCID= en-aut-name=MatanoKazuaki en-aut-sei=Matano en-aut-mei=Kazuaki kn-aut-name= kn-aut-sei= kn-aut-mei= aut-affil-num=6 ORCID= en-aut-name=GuoJing en-aut-sei=Guo en-aut-mei=Jing kn-aut-name= kn-aut-sei= kn-aut-mei= aut-affil-num=7 ORCID= en-aut-name=CaiShu en-aut-sei=Cai en-aut-mei=Shu kn-aut-name= kn-aut-sei= kn-aut-mei= aut-affil-num=8 ORCID= en-aut-name=SunLiling en-aut-sei=Sun en-aut-mei=Liling kn-aut-name= kn-aut-sei= kn-aut-mei= aut-affil-num=9 ORCID= en-aut-name=SarraoJohn L. en-aut-sei=Sarrao en-aut-mei=John L. kn-aut-name= kn-aut-sei= kn-aut-mei= aut-affil-num=10 ORCID= en-aut-name=ThompsonJoe D. en-aut-sei=Thompson en-aut-mei=Joe D. kn-aut-name= kn-aut-sei= kn-aut-mei= aut-affil-num=11 ORCID= en-aut-name=ZhengGuo-Qing en-aut-sei=Zheng en-aut-mei=Guo-Qing kn-aut-name= kn-aut-sei= kn-aut-mei= aut-affil-num=12 ORCID= affil-num=1 en-affil=Department of Physics, Okayama University kn-affil= affil-num=2 en-affil=Department of Physics, Okayama University kn-affil= affil-num=3 en-affil=Department of Physics, Okayama University kn-affil= affil-num=4 en-affil=Department of Physics, Okayama University kn-affil= affil-num=5 en-affil=Department of Physics, Okayama University kn-affil= affil-num=6 en-affil=Department of Physics, Okayama University kn-affil= affil-num=7 en-affil=Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics kn-affil= affil-num=8 en-affil=Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics kn-affil= affil-num=9 en-affil=Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics kn-affil= affil-num=10 en-affil=Los Alamos National Laboratory kn-affil= affil-num=11 en-affil=Los Alamos National Laboratory kn-affil= affil-num=12 en-affil=Department of Physics, Okayama University kn-affil= en-keyword=Condensed-matter physics kn-keyword=Condensed-matter physics en-keyword=Phase transitions and critical phenomena kn-keyword=Phase transitions and critical phenomena en-keyword=Superconducting properties and materials kn-keyword=Superconducting properties and materials END